The old zoo is a great place to hike, and also experience a fun level of creepiness - it's literally an old/abandoned zoo, and you can hike into the former animal enclosures (which now house some pretty impressive layers of graffiti).
Unique things to do nearby
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The Official Hollywood Sign Walking Tour w/ Comedy & Photos
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Private Photoshoot at Popular Locations in LA
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Fabulous views, Hike Runyon Canyon with rescue dogs